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Low tropospheric ozone over the Indo-Pacific Warm Pool related to non-electrified convection

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journal contribution
posted on 2025-04-02, 04:28 authored by Clara M Nussbaumer, Andrea Pozzer, Michael HewsonMichael Hewson, Linda Ort, Bianca Krumm, Joseph Byron, Jonathan Williams, Phillipp Joppe, Florian Obersteiner, Andreas Zahn, Jos Lelieveld, Horst Fischer
Lightning is the most important source of nitric oxide (NO) in the tropical upper troposphere and controls the formation of tropospheric ozone (O3 ${\mathrm{O}}_{3}$). It is associated with deep convection and occurs mostly over continents. The Chemistry of the Atmosphere Field Experiment in the Pacific (CAFE Pacific) was conducted in early 2024 from Cairns, Australia, taking airborne measurements across the Australian continent and the surrounding maritime regions. Based on cloud top properties, lightning data and in situ observations of NO, O3 ${\mathrm{O}}_{3}$ and carbon monoxide, we show that deep convection occurs over Northern Australia and the Indo-Pacific Warm Pool. While we identify strong lightning activity over Australia, we observe deep convection in the Warm Pool that is not electrified. Our observations of low O3 ${\mathrm{O}}_{3}$ in the Warm Pool can be attributed to O3 ${\mathrm{O}}_{3}$-poor air from the marine boundary layer, which is not replenished by photochemical production from NO at high altitudes.

Funding

Category 2 - Other Public Sector Grants Category

History

Volume

52

Issue

5

Start Page

1

End Page

10

Number of Pages

10

eISSN

1944-8007

ISSN

0094-8276

Publisher

American Geophysical Union (AGU)

Additional Rights

CC BY 4.0

Language

en

Peer Reviewed

  • Yes

Open Access

  • Yes

Acceptance Date

2025-02-21

External Author Affiliations

Max Planck Institute for Chemistry

Era Eligible

  • Yes

Journal

Geophysical Research Letters

Article Number

e2024GL112788

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